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Getting set up in Barce with a NIE ??? (Barcelona)

Hi there,
I have EU nationality, and just new in town, apparently obtaining an NIE is the first key admin stepping stone in Barcelona.
Any advice from any of you with EU nationalities as to what the authorities require in terms of official documents to get an NIE and whether it is recommended to pre book a meeting or just show up at the relevant office?
Any tips most appreciated :)

Barcelona Forum