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Recommend a neighborhood to live in? (London)

Hi everyone!

My husband and I will be moving to London in September. He has accepted a position near Cavendish Square Gardens on Henrietta Place. I guess that's the Marylebone area?

We're looking for a lovely, safe neighborhood that isn't too urban, but possesses a good amount of shops, cafes and restaurants. We prefer that the area is within Protected content transportation stops from his workplace (no transfers).

Would you good folks be able to recommend neighborhoods for us to start our flat-renting search? Thanks!

- Mindy